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I am mainly interested in using radiocarbon (14C) to study the biogeochemistry of carbon in aquatic ecosystems (especially large lakes).The temporal (e.g. seasonal) and spatial (depth profile and lateral gradients) distribution of natural abundance 14C signatures of various carbon pools (dissolved organic carbon, particulate organic carbon, dissolved inorganic carbon, particulate inorganic carbon, sedimentary organic carbon) can provide key information on their provenance and biogeochemical transformations. I also use stable isotopes, biomolecular identifiers (biomarkers) and chemical characterization to complement the radiocarbon analysis for a multi-evidence holistic understanding of the cycling of organic carbon.
Below are some specific interests:
- The use of natural abundance bulk 14C content of DOM, and CFRA and CSRA of HMW DOM for constraining sources, average ages and/or residence times and reactivity of organic carbon in aquatic ecosystems.
- The use of bulk and compound-specific stable isotopic signatures (δ13C, δ15N) of DOM and POM for constraining sources and biogeochemical cycling of organic carbon.
- The use of biomarkers (e.g. n-alkanes, sterols) for determining the potential sources of organic carbon in aquatic environments.
- Molecular-level characterization of aquatic DOM using UV-Visible spectroscopy, FTIR spectroscopy, Proton and 13C NMR spectroscopy and ESI-MS.
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